We group together under the above title both the 4d and 5d transition metal ions. The reasons for this are several: the similarities among these elements, at least for our purposes, are much greater than their differences. They also behave distinctly differently from the 3d or iron series ions. Finally, because of expense, synthetic problems and a general lack of an interesting variety of materials to study, there simply has been much less recent research on the magnetochemistry of these elements compared to that on the iron series compounds. Yet, as we shall discuss below, the work at Oxford on the IrX 2-6 ions, for example, has had a profound influence on the subject.
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